Intensification of G/L absorption in microstructured falling film. Application to the treatment of chlorinated VOC's - part II: Modeling and geometric optimization
Identifieur interne : 000C11 ( Main/Exploration ); précédent : 000C10; suivant : 000C12Intensification of G/L absorption in microstructured falling film. Application to the treatment of chlorinated VOC's - part II: Modeling and geometric optimization
Auteurs : Hubert Monnier [France] ; Laurent Falk [France]Source :
- Chemical engineering science [ 0009-2509 ] ; 2011.
Descripteurs français
- Pascal (Inist)
English descriptors
- KwdEn :
Abstract
The falling film microabsorber developed by the Institut für Mikrotechnik Mainz is used to study its performance for the treatment of VOC-containing gases. The technique used is the gas/liquid absorption. The gas (mixture of air and tetrachloroethylene) and the solvent (Di(ethyl-2-hexyl) adipate, DEHA) flow counter-currently in the microabsorber. The solvent streams by gravity on a plate structured by microchannels. This technique makes it possible to miniaturize the process by increasing the mass transfer flow per volume unit as explained in Part I. Experiments are presented and a model is developed from equations of mass and momentum transfers. Results show a competition between two transport phenomena: diffusion and convection. The mass transfer rate is also studied with respect to the structure of microabsorber. It is also shown that it is possible "to optimize" the geometry of the apparatus in order to intensify the transfer so as to miniaturize the process. In the case of physical absorption, mass transfer intensification (Murphree Efficiency) increases when the number of transfer unit NTUG (=τ/ttransfer) increases too. It is mainly due to the small volume of the apparatus where the gas phase residence time must be taken into account in the study of the mass transport towards the gas/liquid interface: the radial and the axial distances for the mass transfer and the mass transport have the same order of magnitude.
Url:
Affiliations:
- France
- Grand Est, Lorraine (région)
- Nancy
- Centre national de la recherche scientifique, Laboratoire réactions et génie des procédés, Université de Lorraine
Links toward previous steps (curation, corpus...)
- to stream PascalFrancis, to step Corpus: 000200
- to stream PascalFrancis, to step Curation: 000911
- to stream PascalFrancis, to step Checkpoint: 000183
- to stream Main, to step Merge: 000D40
- to stream Hal, to step Corpus: 000635
- to stream Hal, to step Curation: 000635
- to stream Hal, to step Checkpoint: 000966
- to stream Main, to step Merge: 000B76
- to stream Main, to step Curation: 000C11
Le document en format XML
<record><TEI><teiHeader><fileDesc><titleStmt><title xml:lang="en" level="a">Intensification of G/L absorption in microstructured falling film. Application to the treatment of chlorinated VOC's - part II: Modeling and geometric optimization</title>
<author><name sortKey="Monnier, Hubert" sort="Monnier, Hubert" uniqKey="Monnier H" first="Hubert" last="Monnier">Hubert Monnier</name>
<affiliation wicri:level="3"><inist:fA14 i1="01"><s1>Nancy University, Laboratory Reactions and Chemical Engineering, LRGP CNRS, 1 rue Grandville</s1>
<s2>54001 Nancy</s2>
<s3>FRA</s3>
<sZ>1 aut.</sZ>
<sZ>2 aut.</sZ>
</inist:fA14>
<country>France</country>
<placeName><region type="region" nuts="2">Grand Est</region>
<region type="old region" nuts="2">Lorraine (région)</region>
<settlement type="city">Nancy</settlement>
</placeName>
</affiliation>
</author>
<author><name sortKey="Falk, Laurent" sort="Falk, Laurent" uniqKey="Falk L" first="Laurent" last="Falk">Laurent Falk</name>
<affiliation wicri:level="3"><inist:fA14 i1="01"><s1>Nancy University, Laboratory Reactions and Chemical Engineering, LRGP CNRS, 1 rue Grandville</s1>
<s2>54001 Nancy</s2>
<s3>FRA</s3>
<sZ>1 aut.</sZ>
<sZ>2 aut.</sZ>
</inist:fA14>
<country>France</country>
<placeName><region type="region" nuts="2">Grand Est</region>
<region type="old region" nuts="2">Lorraine (région)</region>
<settlement type="city">Nancy</settlement>
</placeName>
<placeName><settlement type="city">Nancy</settlement>
<region type="region" nuts="2">Grand Est</region>
<region type="region" nuts="2">Lorraine (région)</region>
</placeName>
<orgName type="laboratoire" n="5">Laboratoire réactions et génie des procédés</orgName>
<orgName type="university">Université de Lorraine</orgName>
<orgName type="institution">Centre national de la recherche scientifique</orgName>
</affiliation>
</author>
</titleStmt>
<publicationStmt><idno type="wicri:source">INIST</idno>
<idno type="inist">11-0242471</idno>
<date when="2011">2011</date>
<idno type="stanalyst">PASCAL 11-0242471 INIST</idno>
<idno type="RBID">Pascal:11-0242471</idno>
<idno type="wicri:Area/PascalFrancis/Corpus">000200</idno>
<idno type="wicri:Area/PascalFrancis/Curation">000911</idno>
<idno type="wicri:Area/PascalFrancis/Checkpoint">000183</idno>
<idno type="wicri:explorRef" wicri:stream="PascalFrancis" wicri:step="Checkpoint">000183</idno>
<idno type="wicri:doubleKey">0009-2509:2011:Monnier H:intensification:of:g</idno>
<idno type="wicri:Area/Main/Merge">000D40</idno>
<idno type="wicri:source">HAL</idno>
<idno type="RBID">Hal:hal-00604834</idno>
<idno type="url">https://hal.archives-ouvertes.fr/hal-00604834</idno>
<idno type="wicri:Area/Hal/Corpus">000635</idno>
<idno type="wicri:Area/Hal/Curation">000635</idno>
<idno type="wicri:Area/Hal/Checkpoint">000966</idno>
<idno type="wicri:explorRef" wicri:stream="Hal" wicri:step="Checkpoint">000966</idno>
<idno type="wicri:doubleKey">0009-2509:2011:Monnier H:intensification:of:g</idno>
<idno type="wicri:Area/Main/Merge">000B76</idno>
<idno type="wicri:Area/Main/Curation">000C11</idno>
<idno type="wicri:Area/Main/Exploration">000C11</idno>
</publicationStmt>
<sourceDesc><biblStruct><analytic><title xml:lang="en" level="a">Intensification of G/L absorption in microstructured falling film. Application to the treatment of chlorinated VOC's - part II: Modeling and geometric optimization</title>
<author><name sortKey="Monnier, Hubert" sort="Monnier, Hubert" uniqKey="Monnier H" first="Hubert" last="Monnier">Hubert Monnier</name>
<affiliation wicri:level="3"><inist:fA14 i1="01"><s1>Nancy University, Laboratory Reactions and Chemical Engineering, LRGP CNRS, 1 rue Grandville</s1>
<s2>54001 Nancy</s2>
<s3>FRA</s3>
<sZ>1 aut.</sZ>
<sZ>2 aut.</sZ>
</inist:fA14>
<country>France</country>
<placeName><region type="region" nuts="2">Grand Est</region>
<region type="old region" nuts="2">Lorraine (région)</region>
<settlement type="city">Nancy</settlement>
</placeName>
</affiliation>
</author>
<author><name sortKey="Falk, Laurent" sort="Falk, Laurent" uniqKey="Falk L" first="Laurent" last="Falk">Laurent Falk</name>
<affiliation wicri:level="3"><inist:fA14 i1="01"><s1>Nancy University, Laboratory Reactions and Chemical Engineering, LRGP CNRS, 1 rue Grandville</s1>
<s2>54001 Nancy</s2>
<s3>FRA</s3>
<sZ>1 aut.</sZ>
<sZ>2 aut.</sZ>
</inist:fA14>
<country>France</country>
<placeName><region type="region" nuts="2">Grand Est</region>
<region type="old region" nuts="2">Lorraine (région)</region>
<settlement type="city">Nancy</settlement>
</placeName>
<placeName><settlement type="city">Nancy</settlement>
<region type="region" nuts="2">Grand Est</region>
<region type="region" nuts="2">Lorraine (région)</region>
</placeName>
<orgName type="laboratoire" n="5">Laboratoire réactions et génie des procédés</orgName>
<orgName type="university">Université de Lorraine</orgName>
<orgName type="institution">Centre national de la recherche scientifique</orgName>
</affiliation>
</author>
</analytic>
<series><title level="j" type="main">Chemical engineering science</title>
<title level="j" type="abbreviated">Chem. eng. sci.</title>
<idno type="ISSN">0009-2509</idno>
<imprint><date when="2011">2011</date>
</imprint>
</series>
</biblStruct>
</sourceDesc>
<seriesStmt><title level="j" type="main">Chemical engineering science</title>
<title level="j" type="abbreviated">Chem. eng. sci.</title>
<idno type="ISSN">0009-2509</idno>
</seriesStmt>
</fileDesc>
<profileDesc><textClass><keywords scheme="KwdEn" xml:lang="en"><term>Convection</term>
<term>Diffusion</term>
<term>Falling film</term>
<term>Gas liquid interface</term>
<term>Gas mixture</term>
<term>Mass transfer</term>
<term>Modeling</term>
<term>Momentum transfer</term>
<term>Murphree efficiency</term>
<term>Optimization</term>
<term>Physisorption</term>
<term>Transport process</term>
<term>Volatile organic compound</term>
</keywords>
<keywords scheme="Pascal" xml:lang="fr"><term>Film tombant</term>
<term>Composé organique volatil</term>
<term>Modélisation</term>
<term>Optimisation</term>
<term>Mélange gaz</term>
<term>Transfert masse</term>
<term>Transfert quantité mouvement</term>
<term>Phénomène transport</term>
<term>Diffusion</term>
<term>Convection</term>
<term>Physisorption</term>
<term>Efficacité Murphree</term>
<term>Interface gaz liquide</term>
</keywords>
</textClass>
</profileDesc>
</teiHeader>
<front><div type="abstract" xml:lang="en">The falling film microabsorber developed by the Institut für Mikrotechnik Mainz is used to study its performance for the treatment of VOC-containing gases. The technique used is the gas/liquid absorption. The gas (mixture of air and tetrachloroethylene) and the solvent (Di(ethyl-2-hexyl) adipate, DEHA) flow counter-currently in the microabsorber. The solvent streams by gravity on a plate structured by microchannels. This technique makes it possible to miniaturize the process by increasing the mass transfer flow per volume unit as explained in Part I. Experiments are presented and a model is developed from equations of mass and momentum transfers. Results show a competition between two transport phenomena: diffusion and convection. The mass transfer rate is also studied with respect to the structure of microabsorber. It is also shown that it is possible "to optimize" the geometry of the apparatus in order to intensify the transfer so as to miniaturize the process. In the case of physical absorption, mass transfer intensification (Murphree Efficiency) increases when the number of transfer unit NTU<sub>G</sub>
(=τ/t<sub>transfer</sub>
) increases too. It is mainly due to the small volume of the apparatus where the gas phase residence time must be taken into account in the study of the mass transport towards the gas/liquid interface: the radial and the axial distances for the mass transfer and the mass transport have the same order of magnitude.</div>
</front>
</TEI>
<affiliations><list><country><li>France</li>
</country>
<region><li>Grand Est</li>
<li>Lorraine (région)</li>
</region>
<settlement><li>Nancy</li>
</settlement>
<orgName><li>Centre national de la recherche scientifique</li>
<li>Laboratoire réactions et génie des procédés</li>
<li>Université de Lorraine</li>
</orgName>
</list>
<tree><country name="France"><region name="Grand Est"><name sortKey="Monnier, Hubert" sort="Monnier, Hubert" uniqKey="Monnier H" first="Hubert" last="Monnier">Hubert Monnier</name>
</region>
<name sortKey="Falk, Laurent" sort="Falk, Laurent" uniqKey="Falk L" first="Laurent" last="Falk">Laurent Falk</name>
</country>
</tree>
</affiliations>
</record>
Pour manipuler ce document sous Unix (Dilib)
EXPLOR_STEP=$WICRI_ROOT/Wicri/Lorraine/explor/LrgpV1/Data/Main/Exploration
HfdSelect -h $EXPLOR_STEP/biblio.hfd -nk 000C11 | SxmlIndent | more
Ou
HfdSelect -h $EXPLOR_AREA/Data/Main/Exploration/biblio.hfd -nk 000C11 | SxmlIndent | more
Pour mettre un lien sur cette page dans le réseau Wicri
{{Explor lien |wiki= Wicri/Lorraine |area= LrgpV1 |flux= Main |étape= Exploration |type= RBID |clé= Pascal:11-0242471 |texte= Intensification of G/L absorption in microstructured falling film. Application to the treatment of chlorinated VOC's - part II: Modeling and geometric optimization }}
This area was generated with Dilib version V0.6.32. |